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    Global Temperature Dependency of Biogenic HCHO Columns Observed From Space: Interpretation of TROPOMI Results Using GEOS-Chem Model

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    Authors
    Li, X.
    Zhu, L.
    De Smedt, I.
    Sun, W.
    Chen, Y.
    Shu, L.
    Wang, D.
    Liu, S.
    Pu, D.
    Li, J.
    Zuo, X.
    Fu, W.
    Li, Y.
    Zhang, P.
    Yan, Z.
    Fu, T.-M.
    Shen, H.
    Wang, C.
    Ye, J.
    Yang, X.
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    Discipline
    Earth and related Environmental sciences
    Subject
    TROPOMI
    HCHO
    BVOC
    temperature dependency
    GEOS-Chem
    MEGAN
    Audience
    Scientific
    Date
    2024
    Metadata
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    Description
    Temperature is the principal driver of global atmospheric formaldehyde (HCHO) and its primary oxidation precursor biogenic volatile organic compounds (BVOCs). We revisit such a temperature (T-) dependency globally, leveraging TROPOMI HCHO column data. We find substantial variations in the T-dependency of biogenic HCHO across plant functional types (PFTs), with the highest over Broadleaf Evergreen Tropical Trees (doubling every 6.0 K ± 4.1 K) and lowest over Arctic C3 Grass (doubling every 30.8 K ± 9.6 K). The GEOS-Chem model interprets HCHO columns' T-dependency at the PFT level (r = 0.87), with a 16% discrepancy on average. The discrepancy can be explained by BVOC emissions T-dependency for Broadleaf Evergreen Tropical Trees and Warm C4 Grass and can be attributed to the insensitivity of HCHO columns to BVOC emissions for other PFTs. Our findings underscore a potentially magnified variation of BVOC emissions by GEOS-Chem and MEGAN therein, particularly in regions experiencing greater temperature variations.
    Citation
    Li, X.; Zhu, L.; De Smedt, I.; Sun, W.; Chen, Y.; Shu, L.; Wang, D.; Liu, S.; Pu, D.; Li, J.; Zuo, X.; Fu, W.; Li, Y.; Zhang, P.; Yan, Z.; Fu, T.-M.; Shen, H.; Wang, C.; Ye, J.; Yang, X. (2024). Global Temperature Dependency of Biogenic HCHO Columns Observed From Space: Interpretation of TROPOMI Results Using GEOS-Chem Model. , Journal of Geophysical Research: Atmospheres, Vol. 129, Issue 21, e2024JD041784, DOI: 10.1029/2024JD041784.
    Identifiers
    uri: https://orfeo.belnet.be/handle/internal/13522
    doi: http://dx.doi.org/10.1029/2024JD041784
    url:
    Type
    Article
    Peer-Review
    Yes
    Language
    eng
    Links
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