Global Temperature Dependency of Biogenic HCHO Columns Observed From Space: Interpretation of TROPOMI Results Using GEOS-Chem Model
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Authors
Li, X.
Zhu, L.
De Smedt, I.
Sun, W.
Chen, Y.
Shu, L.
Wang, D.
Liu, S.
Pu, D.
Li, J.
Zuo, X.
Fu, W.
Li, Y.
Zhang, P.
Yan, Z.
Fu, T.-M.
Shen, H.
Wang, C.
Ye, J.
Yang, X.
Discipline
Earth and related Environmental sciences
Subject
TROPOMI
HCHO
BVOC
temperature dependency
GEOS-Chem
MEGAN
Audience
Scientific
Date
2024Metadata
Show full item recordDescription
Temperature is the principal driver of global atmospheric formaldehyde (HCHO) and its primary oxidation precursor biogenic volatile organic compounds (BVOCs). We revisit such a temperature (T-) dependency globally, leveraging TROPOMI HCHO column data. We find substantial variations in the T-dependency of biogenic HCHO across plant functional types (PFTs), with the highest over Broadleaf Evergreen Tropical Trees (doubling every 6.0 K ± 4.1 K) and lowest over Arctic C3 Grass (doubling every 30.8 K ± 9.6 K). The GEOS-Chem model interprets HCHO columns' T-dependency at the PFT level (r = 0.87), with a 16% discrepancy on average. The discrepancy can be explained by BVOC emissions T-dependency for Broadleaf Evergreen Tropical Trees and Warm C4 Grass and can be attributed to the insensitivity of HCHO columns to BVOC emissions for other PFTs. Our findings underscore a potentially magnified variation of BVOC emissions by GEOS-Chem and MEGAN therein, particularly in regions experiencing greater temperature variations.
Citation
Li, X.; Zhu, L.; De Smedt, I.; Sun, W.; Chen, Y.; Shu, L.; Wang, D.; Liu, S.; Pu, D.; Li, J.; Zuo, X.; Fu, W.; Li, Y.; Zhang, P.; Yan, Z.; Fu, T.-M.; Shen, H.; Wang, C.; Ye, J.; Yang, X. (2024). Global Temperature Dependency of Biogenic HCHO Columns Observed From Space: Interpretation of TROPOMI Results Using GEOS-Chem Model. , Journal of Geophysical Research: Atmospheres, Vol. 129, Issue 21, e2024JD041784, DOI: 10.1029/2024JD041784.Identifiers
url:
Type
Article
Peer-Review
Yes
Language
eng