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    A global inventory of stratospheric NOy from ACE-FTS

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    Authors
    Jones, A.
    Qin, G.
    Strong, K.
    Walker, K.A.
    McLinden, C.A.
    Toohey, M.
    Kerzenmacher, T.
    Bernath, P.F.
    Boone, C.D.
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    Discipline
    Earth and related Environmental sciences
    Subject
    Atmospheric chemistry
    Atmospherics
    Budget control
    Climatology
    Fourier transforms
    Nitric acid
    Nitrogen
    ACE-FTS
    Atmospheric chemistry experiment
    Atmospheric species
    Data sets
    Denitrification process
    Energetic particles
    Fourier transform spectrometers
    Global inventories
    Heterogeneous chemistry
    Midlatitudes
    Polar Regions
    Polar vortex
    Pressure surface
    SCISAT-1
    Trace-gases
    Volume mixing ratios
    Spacecraft instruments
    ACE 1
    atmospheric chemistry
    atmospheric transport
    climatology
    concentration (composition)
    data set
    denitrification
    FTIR spectroscopy
    inventory
    mesosphere
    mixing ratio
    nitrous oxide
    polar region
    polar vortex
    pressure field
    satellite imagery
    stratosphere
    trace gas
    World Wide Web
    Audience
    Scientific
    Date
    2011
    Metadata
    Show full item record
    Description
    The Atmospheric Chemistry Experiment Fourier Transform Spectrometer (ACE-FTS) on board the Canadian SCISAT-1 satellite (launched in August 2003) measures over 30 different atmospheric species, including six nitrogen trace gases that are needed to quantify the stratospheric NOy budget. We combine volume mixing ratio (VMR) profiles for NO, NO2, HNO3, N2O5, ClONO2, and HNO4 to determine a zonally averaged NOy climatology on monthly and 3 month combined means (December–February, March–May, June–August, and September–November) at 5° latitude spacing and on 33 pressure surfaces. Peak NOy VMR concentrations (15–20 ppbv) are situated at about 3 hPa (∼40 km) in the tropics, while they are typically lower at about 10 hPa (∼30 km) in the midlatitudes. Mean NOy VMRs are similar in both the northern and southern polar regions, with the exception of large enhancements periodically observed in the upper stratosphere and lower mesosphere. These are primarily due to enhancements of NO due to energetic particle precipitation and downward transport. Other features in the NOy budget are related to descent in the polar vortex, heterogeneous chemistry, and denitrification processes. Comparison of the ACE-FTS NOy budget is made to both the Odin and ATMOS NOy data sets, showing in both cases a good level of agreement, such that relative differences are typically better than 20%. The NOy climatological products are available through the ACE website and are a supplement to the paper.
    Citation
    Jones, A.; Qin, G.; Strong, K.; Walker, K.A.; McLinden, C.A.; Toohey, M.; Kerzenmacher, T.; Bernath, P.F.; Boone, C.D. (2011). A global inventory of stratospheric NOy from ACE-FTS. , Journal of Geophysical Research: Atmospheres, Vol. 116, Issue 17, D17304, DOI: 10.1029/2010JD015465.
    Identifiers
    uri: https://orfeo.belnet.be/handle/internal/3087
    doi: http://dx.doi.org/10.1029/2010JD015465
    Type
    Article
    Peer-Review
    Yes
    Language
    eng
    Links
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