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    One-decade trend analysis of stratospheric BrO over Harestua (60°N) and Lauder (45°S) reveals a decline

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    Authors
    Hendrick, F.
    Johnston, P.V.
    De Mazière, M.
    Fayt, C.
    Hermans, C.
    Kreher, K.
    Theys, N.
    Thomas, A.
    Van Roozendael, M.
    Show allShow less
    Discipline
    Physical sciences
    Subject
    Network protocols
    Sulfur compounds
    Troposphere
    Brominated substances
    Ground-based
    Inorganic bromine
    Mean age of air
    Montreal protocol
    Trend analysis
    Uv-visible
    Very short-lived substances
    Bromine
    air quality
    atmospheric chemistry
    bromine
    decadal variation
    ground-based measurement
    Montreal Protocol
    stratosphere
    trend analysis
    troposphere
    Australasia
    Eurasia
    Europe
    Harestua
    Lauder
    New Zealand
    Northern Europe
    Norway
    Oppland
    Otago
    Scandinavia
    South Island
    Audience
    Scientific
    Date
    2008
    Metadata
    Show full item record
    Description
    A trend analysis is performed of stratospheric BrO from ground-based UV-visible observations at Harestua (60°N, 11°E) and Lauder (45°S, 170°E) from 1995 through 2005. At both stations, a positive trend of about +2.5% per year is found for the 1995-2001 period, while a negative trend of about -1% per year is obtained between 2001 and 2005. Given a mean age of air of about 4 ± 1 years, the decline in stratospheric bromine since 2002 follows the decline of tropospheric organic bromine observed since the second half of 1998, as a result of the Montreal Protocol. These findings confirm that the impact of the Montreal Protocol restrictions on brominated substances have now reached the stratosphere. From our study, we have also derived a contribution of 6 ± 4 ppt of the brominated very short-lived substances and inorganic bromine tropospheric sources to the total bromine loading.
    Citation
    Hendrick, F.; Johnston, P.V.; De Mazière, M.; Fayt, C.; Hermans, C.; Kreher, K.; Theys, N.; Thomas, A.; Van Roozendael, M. (2008). One-decade trend analysis of stratospheric BrO over Harestua (60°N) and Lauder (45°S) reveals a decline. , Geophysical Research Letters, Vol. 35, Issue 14, L14801, DOI: 10.1029/2008GL034154.
    Identifiers
    uri: https://orfeo.belnet.be/handle/internal/4323
    doi: http://dx.doi.org/10.1029/2008GL034154
    scopus: 2-s2.0-53749083832
    Type
    Article
    Peer-Review
    Yes
    Language
    eng
    Links
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