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    Validation of NO2 and NO from the Atmospheric Chemistry Experiment (ACE)

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    Authors
    Kerzenmacher, T.
    Wolff, M.A.
    Strong, K.
    Dupuy, E.
    Walker, K.A.
    Amekudzi, L.K.
    Batchelor, R.L.
    Bernath, P.F.
    Berthet, G.
    Blumenstock, T.
    Boone, C.D.
    Bramstedt, K.
    Brogniez, C.
    Brohede, S.
    Burrows, J.P.
    Catoire, V.
    Dodion, J.
    Drummond, J.R.
    Dufour, D.G.
    Funke, B.
    Fussen, D.
    Goutail, F.
    Griffith, D.W.T.
    Haley, C.S.
    Hendrick, F.
    Höpfner, M.
    Huret, N.
    Jones, N.
    Kar, J.
    Kramer, I.
    Llewellyn, E.J.
    López-Puertas, M.
    Manney, G.
    McElroy, C.T.
    McLinden, C.A.
    Melo, S.
    Mikuteit, S.
    Murtagh, D.
    Nichitiu, F.
    Notholt, J.
    Nowlan, C.
    Piccolo, C.
    Pommereau, J.-P.
    Randall, C.
    Raspollini, P.
    Ridolfi, M.
    Richter, A.
    Schneider, M.
    Schrems, O.
    Silicani, M.
    Stiller, G.P.
    Taylor, J.
    Tétard, C.
    Toohey, M.
    Vanhellemont, F.
    Warneke, T.
    Zawodny, J.M.
    Zou, J.
    Show allShow less
    Discipline
    Physical sciences
    Subject
    ACE 1
    comparative study
    mixing ratio
    nitrogen dioxide
    nitrogen oxides
    satellite data
    spectrometer
    Audience
    Scientific
    Date
    2008
    Metadata
    Show full item record
    Description
    Vertical profiles of NO2 and NO have been obtained from solar occultation measurements by the Atmospheric Chemistry Experiment (ACE), using an infrared Fourier Transform Spectrometer (ACE-FTS) and (for NO2) an ultraviolet-visible-near-infrared spectrometer, MAESTRO (Measurement of Aerosol Extinction in the Stratosphere and Troposphere Retrieved by Occultation). In this paper, the quality of the ACE-FTS version 2.2 NO2 and NO and the MAESTRO version 1.2 NO2 data are assessed using other solar occultation measurements (HALOE, SAGE II, SAGE III, POAM III, SCIAMACHY), stellar occultation measurements (GOMOS), limb measurements (MIPAS, OSIRIS), nadir measurements (SCIAMACHY), balloon-borne measurements (SPIRALE, SAOZ) and ground-based measurements (UV-VIS, FTIR). Time differences between the comparison measurements were reduced using either a tight coincidence criterion, or where possible, chemical box models. ACE-FTS NO2 and NO and the MAESTRO NO2 are generally consistent with the correlative data. The ACE-FTS and MAESTRO NO2 volume mixing ratio (VMR) profiles agree with the profiles from other satellite data sets to within about 20% between 25 and 40 km, with the exception of MIPAS ESA (for ACE-FTS) and SAGE II (for ACE-FTS (sunrise) and MAESTRO) and suggest a negative bias between 23 and 40 km of about 10%. MAESTRO reports larger VMR values than the ACE-FTS. In comparisons with HALOE, ACE-FTS NO VMRs typically (on average) agree to ±8% from 22 to 64 km and to +10% from 93 to 105 km, with maxima of 21% and 36%, respectively. Partial column comparisons for NO2 show that there is quite good agreement between the ACE instruments and the FTIRs, with a mean difference of +7.3% for ACE-FTS and +12.8% for MAESTRO.
    Citation
    Kerzenmacher, T.; Wolff, M.A.; Strong, K.; Dupuy, E.; Walker, K.A.; Amekudzi, L.K.; Batchelor, R.L.; Bernath, P.F.; Berthet, G.; Blumenstock, T.; Boone, C.D.; Bramstedt, K.; Brogniez, C.; Brohede, S.; Burrows, J.P.; Catoire, V.; Dodion, J.; Drummond, J.R.; Dufour, D.G.; Funke, B.; Fussen, D.; Goutail, F.; Griffith, D.W.T.; Haley, C.S.; Hendrick, F.; Höpfner, M.; Huret, N.; Jones, N.; Kar, J.; Kramer, I.; Llewellyn, E.J.; López-Puertas, M.; Manney, G.; McElroy, C.T.; McLinden, C.A.; Melo, S.; Mikuteit, S.; Murtagh, D.; Nichitiu, F.; Notholt, J.; Nowlan, C.; Piccolo, C.; Pommereau, J.-P.; Randall, C.; Raspollini, P.; Ridolfi, M.; Richter, A.; Schneider, M.; Schrems, O.; Silicani, M.; Stiller, G.P.; Taylor, J.; Tétard, C.; Toohey, M.; Vanhellemont, F.; Warneke, T.; Zawodny, J.M.; Zou, J. (2008). Validation of NO2 and NO from the Atmospheric Chemistry Experiment (ACE). , Atmospheric Chemistry and Physics, Vol. 8, Issue 19, 5801-5841, DOI: 10.5194/acp-8-5801-2008.
    Identifiers
    uri: https://orfeo.belnet.be/handle/internal/4352
    doi: http://dx.doi.org/10.5194/acp-8-5801-2008
    scopus: 2-s2.0-54049157508
    Type
    Article
    Peer-Review
    Yes
    Language
    eng
    Links
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