Intercomparison of BrO measurements from ERS-2 GOME, ground-based and balloon platforms
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Authors
Van Roozendael, M.
Wagner, T.
Richter, A.
Pundt, I.
Arlander, D.W.
Burrows, J.P.
Chipperfield, M.
Fayt, C.
Johnston, P.V.
Lambert, J.-C.
Kreher, K.
Pfeilsticker, K.
Platt, U.
Pommereau, J.-P.
Sinnhuber, B.-M.
Tornkvist, K.K.
Wittrock, F.
Discipline
Physical sciences
Subject
Bromine compounds
Meteorological balloons
Ozone
Troposphere
Latitudes
Space research
balloon observation
bromide
ERS-2
GOME
ground-based measurement
zenith angle
Audience
Scientific
Date
2002Metadata
Show full item recordDescription
The consistency of BrO column amounts derived from GOME spectra and from correlative ground-based and balloon measurements performed in 1998-1999 during the Third European Stratospheric Experiment on Ozone (THESEO) has been investigated. The study relies on UV-visible observations at several mid- and high latitude ground-based stations in both hemispheres, complemented by balloon-borne solar occultation profile measurements and 3D chemical transport model simulations. Previous investigations have reported GOME BrO columns systematically larger than those deduced from balloon, suggesting BrO being present, possibly ubiquitously, in the free troposphere. The robustness of this hypothesis has been further tested based on the presently available correlative data set. It is shown that when accounting for the BrO diurnal variation and the solar zenith angle dependency of the sensitivity of correlative data to the troposphere, measurements from all platforms are consistent with the presence of a tropospheric BrO background of 1-3 × 1013 molec/cm2 extending over mid- and high latitudes.
Citation
Van Roozendael, M.; Wagner, T.; Richter, A.; Pundt, I.; Arlander, D.W.; Burrows, J.P.; Chipperfield, M.; Fayt, C.; Johnston, P.V.; Lambert, J.-C.; Kreher, K.; Pfeilsticker, K.; Platt, U.; Pommereau, J.-P.; Sinnhuber, B.-M.; Tornkvist, K.K.; Wittrock, F. (2002). Intercomparison of BrO measurements from ERS-2 GOME, ground-based and balloon platforms. , Advances in Space Research, Vol. 29, Issue 11, 1661-1666, DOI: 10.1016/S0273-1177(02)00098-4.Identifiers
scopus: 2-s2.0-6444244778
Type
Article
Peer-Review
Yes
Language
eng