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    Radiative forcing due to increased tropospheric ozone concentrations

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    Chalita(1996a).pdf (501.5Kb)
    Authors
    Chalita, S.
    Hauglustaine, D.A.
    Le Treut, H.
    Müller, J.-F.
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    Discipline
    Earth and related Environmental sciences
    Subject
    ozone
    boundary layer
    conference paper
    geographic distribution
    priority journal
    seasonal variation
    solar radiation
    summer
    troposphere
    Boundary layers
    Computer simulation
    Infrared radiation
    Mathematical models
    Sensitivity analysis
    Solar radiation
    Three dimensional
    Troposphere
    General circulation model
    Northern hemisphere
    Radiative forcing
    Ozone
    chemistry transport model
    GCM
    IMAGES
    LMD GCM
    model
    ozone
    radiative forcing
    troposphere
    Audience
    Scientific
    Date
    1996
    Metadata
    Show full item record
    Description
    Increasing tropospheric ozone concentrations have been observed in the past decades in industrialized and remote areas of the Northern Hemisphere. Since ozone absorbs both solar and infrared radiation, several studies concerning the tropospheric ozone-climate problem have been recently conducted mainly with one- and two-dimensional models. In this study, pre-industrial and present-day tropospheric ozone concentrations simulated by a three-dimensional Chemistry Transport Model (3-D CTM) IMAGES (Intermediate Model for the Annual and Global Evolution of Species) are used in conjunction with the Laboratoire de Meteorologie Dynamique General Circulation Model (LMD GCM) to determine the ozone radiative forcing since the pre-industrial era. We find that the ozone forcing is regionally heterogeneous with a marked interhemispheric difference and a strong seasonal variation, peaking over the Northern Hemisphere continents during summer and reaching locally more than 1 Wm-2. Sensitivity simulations confirm that the major contributions to the tropopause forcing arise from ozone changes occurring in the high troposphere. Changes of ozone concentration in the planetary boundary layer are about 10 times less efficient than in the high troposphere in terms of radiative perturbation. These 3D results also confirm the quasi-linear relationship between the radiative forcing and the tropospheric ozone increase for both hemispheres. Some previsions of future forcing change considering a critical constant global rate of ozone increase equal to 10% per decade and the IS92a IPCC emission scenario are realized for the next century.
    Citation
    Chalita, S.; Hauglustaine, D.A.; Le Treut, H.; Müller, J.-F. (1996). Radiative forcing due to increased tropospheric ozone concentrations. , Atmospheric Environment, Vol. 30, Issue 10-11, 1641-1646, DOI: 10.1016/1352-2310(95)00431-9.
    Identifiers
    uri: https://orfeo.belnet.be/handle/internal/5497
    doi: http://dx.doi.org/10.1016/1352-2310(95)00431-9
    scopus: 2-s2.0-0029663084
    Type
    Article
    Peer-Review
    Yes
    Language
    eng
    Links
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