• Login
     
    View Item 
    •   ORFEO Home
    • Royal Belgian Institute for Space Aeronomy
    • BIRA-IASB publications
    • View Item
    •   ORFEO Home
    • Royal Belgian Institute for Space Aeronomy
    • BIRA-IASB publications
    • View Item
    JavaScript is disabled for your browser. Some features of this site may not work without it.

    Updated SO2 emission estimates over China using OMI/Aura observations

    Thumbnail
    View/Open
    Koukouli(2018a).pdf (3.786Mb)
    Authors
    Koukouli, M.E.
    Theys, N.
    Ding, J.
    Zyrichidou, I.
    Mijling, B.
    Balis, D.
    Van der A, R.J.
    Show allShow less
    Discipline
    Earth and related Environmental sciences
    Audience
    Scientific
    Date
    2018
    Metadata
    Show full item record
    Description
    The main aim of this paper is to update existing sulfur dioxide (SO2) emission inventories over China using modern inversion techniques, state-of-the-art chemistry transport modelling (CTM) and satellite observations of SO2. Within the framework of the EU Seventh Framework Programme (FP7) MarcoPolo (Monitoring and Assessment of Regional air quality in China using space Observations) project, a new SO2 emission inventory over China was calculated using the CHIMERE v2013b CTM simulations, 10 years of Ozone Monitoring Instrument (OMI)/Aura total SO2 columns and the pre-existing Multi-resolution Emission Inventory for China (MEIC v1.2). It is shown that including satellite observations in the calculations increases the current bottom-up MEIC inventory emissions for the entire domain studied (15–55° N, 102–132° E) from 26.30 to 32.60 Tg annum−1, with positive updates which are stronger in winter ( ∼  36 % increase). New source areas were identified in the southwest (25–35° N, 100–110° E) as well as in the northeast (40–50° N, 120–130° E) of the domain studied as high SO2 levels were observed by OMI, resulting in increased emissions in the a posteriori inventory that do not appear in the original MEIC v1.2 dataset. Comparisons with the independent Emissions Database for Global Atmospheric Research, EDGAR v4.3.1, show a satisfying agreement since the EDGAR 2010 bottom-up database provides 33.30 Tg annum−1 of SO2 emissions. When studying the entire OMI/Aura time period (2005 to 2015), it was shown that the SO2 emissions remain nearly constant before the year 2010, with a drift of −0.51 ± 0.38 Tg annum−1, and show a statistically significant decline after the year 2010 of −1.64 ± 0.37 Tg annum−1 for the entire domain. Similar findings were obtained when focusing on the greater Beijing area (30–40° N, 110–120° E) with pre-2010 drifts of −0.17 ± 0.14 and post-2010 drifts of −0.47 ± 0.12 Tg annum−1. The new SO2 emission inventory is publicly available and forms part of the official EU MarcoPolo emission inventory over China, which also includes updated NOx, volatile organic compounds and particulate matter emissions.
    Citation
    Koukouli, M.E.; Theys, N.; Ding, J.; Zyrichidou, I.; Mijling, B.; Balis, D.; Van der A, R.J. (2018). Updated SO2 emission estimates over China using OMI/Aura observations. , Atmospheric Measurement Techniques, Vol. 11, Issue 3, 1817-1832, DOI: 10.5194/amt-11-1817-2018.
    Identifiers
    uri: https://orfeo.belnet.be/handle/internal/6896
    doi: http://dx.doi.org/10.5194/amt-11-1817-2018
    Type
    Article
    Peer-Review
    Yes
    Language
    eng
    Links
    NewsHelpdeskBELSPO OA Policy

    Browse

    All of ORFEOCommunities & CollectionsBy Issue DateAuthorsTitlesDisciplinesThis CollectionBy Issue DateAuthorsTitlesDisciplines
     

    DSpace software copyright © 2002-2016  DuraSpace
    Send Feedback | Cookie Information
    Theme by 
    Atmire NV